IRIS publication 16860761
Effect of magnetic defects and dimensionality on the spin dynamics of GeMn systems: Electron spin resonance measurements
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TY - JOUR - Kazakova, O.,Morgunov, R.,Kulkarni, J.,Holmes, J.,Ottaviano, L. - 2008 - June - Physical Review B - Effect of magnetic defects and dimensionality on the spin dynamics of GeMn systems: Electron spin resonance measurements - Validated - () - 77 - 23 - Effects of dimensionality on magnetic and electric properties of one- and two-dimensional GeMn systems and the role of defects in magnetic ordering are investigated by means of electron spin resonance (ESR) and superconducting quantum interference device magnetometry techniques. Arrays of Ge1-xMnx nanowires and thin Ge:Mn films with similar concentrations of the magnetic impurity (x=1%-8%) have been fabricated by chemical synthesis and ion implantation, respectively. In magnetically homogeneous Ge1-xMnx nanowires, all observed electron spin resonances are related to absorption on individual magnetic centers (Mn3+ and Mn2+ ions and polarized charge carriers) in a broad temperature range, T=5-300 K. On the other hand, in strongly inhomogeneous 2D GeMn films, a collective spin excitation, the spin-wave resonance, is observed at low temperatures, T=5-60 K. This signifies the presence of long-range spin states and a cooperative magnetic response originating from crystalline Mn5Ge3 precipitates and Mn-rich amorphous nanoclusters as well as diluted Mn ions. Additionally, a strong negative background was observed and attributed to the microwave magnetoresistance of the Ge:Mn thin films. The absence of the magnetoresistance in Ge1-xMnx nanowires indicates that the scattering of charge carriers is determined by dimensions of the structure. Overall, our analysis of magnetic-resonance phenomena reveals a significant difference between one-dimensional and two-dimensional magnetic semiconductors. It emphasizes the important role of dimensionality as well as the type and distribution of magnetic defects in spin-dependent scattering and dynamic magnetic properties of GeMn semiconductors. - 1098-0121 - ://000257289500084 DA - 2008/06 ER -
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@article{V16860761, = {Kazakova, O. and Morgunov, R. and Kulkarni, J. and Holmes, J. and Ottaviano, L. }, = {2008}, = {June}, = {Physical Review B}, = {Effect of magnetic defects and dimensionality on the spin dynamics of GeMn systems: Electron spin resonance measurements}, = {Validated}, = {()}, = {77}, = {23}, = {{Effects of dimensionality on magnetic and electric properties of one- and two-dimensional GeMn systems and the role of defects in magnetic ordering are investigated by means of electron spin resonance (ESR) and superconducting quantum interference device magnetometry techniques. Arrays of Ge1-xMnx nanowires and thin Ge:Mn films with similar concentrations of the magnetic impurity (x=1%-8%) have been fabricated by chemical synthesis and ion implantation, respectively. In magnetically homogeneous Ge1-xMnx nanowires, all observed electron spin resonances are related to absorption on individual magnetic centers (Mn3+ and Mn2+ ions and polarized charge carriers) in a broad temperature range, T=5-300 K. On the other hand, in strongly inhomogeneous 2D GeMn films, a collective spin excitation, the spin-wave resonance, is observed at low temperatures, T=5-60 K. This signifies the presence of long-range spin states and a cooperative magnetic response originating from crystalline Mn5Ge3 precipitates and Mn-rich amorphous nanoclusters as well as diluted Mn ions. Additionally, a strong negative background was observed and attributed to the microwave magnetoresistance of the Ge:Mn thin films. The absence of the magnetoresistance in Ge1-xMnx nanowires indicates that the scattering of charge carriers is determined by dimensions of the structure. Overall, our analysis of magnetic-resonance phenomena reveals a significant difference between one-dimensional and two-dimensional magnetic semiconductors. It emphasizes the important role of dimensionality as well as the type and distribution of magnetic defects in spin-dependent scattering and dynamic magnetic properties of GeMn semiconductors.}}, issn = {1098-0121}, = {://000257289500084}, source = {IRIS} }
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AUTHORS | Kazakova, O.,Morgunov, R.,Kulkarni, J.,Holmes, J.,Ottaviano, L. | ||
YEAR | 2008 | ||
MONTH | June | ||
JOURNAL_CODE | Physical Review B | ||
TITLE | Effect of magnetic defects and dimensionality on the spin dynamics of GeMn systems: Electron spin resonance measurements | ||
STATUS | Validated | ||
TIMES_CITED | () | ||
SEARCH_KEYWORD | |||
VOLUME | 77 | ||
ISSUE | 23 | ||
START_PAGE | |||
END_PAGE | |||
ABSTRACT | Effects of dimensionality on magnetic and electric properties of one- and two-dimensional GeMn systems and the role of defects in magnetic ordering are investigated by means of electron spin resonance (ESR) and superconducting quantum interference device magnetometry techniques. Arrays of Ge1-xMnx nanowires and thin Ge:Mn films with similar concentrations of the magnetic impurity (x=1%-8%) have been fabricated by chemical synthesis and ion implantation, respectively. In magnetically homogeneous Ge1-xMnx nanowires, all observed electron spin resonances are related to absorption on individual magnetic centers (Mn3+ and Mn2+ ions and polarized charge carriers) in a broad temperature range, T=5-300 K. On the other hand, in strongly inhomogeneous 2D GeMn films, a collective spin excitation, the spin-wave resonance, is observed at low temperatures, T=5-60 K. This signifies the presence of long-range spin states and a cooperative magnetic response originating from crystalline Mn5Ge3 precipitates and Mn-rich amorphous nanoclusters as well as diluted Mn ions. Additionally, a strong negative background was observed and attributed to the microwave magnetoresistance of the Ge:Mn thin films. The absence of the magnetoresistance in Ge1-xMnx nanowires indicates that the scattering of charge carriers is determined by dimensions of the structure. Overall, our analysis of magnetic-resonance phenomena reveals a significant difference between one-dimensional and two-dimensional magnetic semiconductors. It emphasizes the important role of dimensionality as well as the type and distribution of magnetic defects in spin-dependent scattering and dynamic magnetic properties of GeMn semiconductors. | ||
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ISBN_ISSN | 1098-0121 | ||
EDITION | |||
URL | ://000257289500084 | ||
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