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Dichotomous dynamics of magnetic monopole fluids

  • Chun Chih Hsu
  • , Hiroto Takahashi
  • , Fabian Jerzembeck
  • , Jahnatta Dasini
  • , Chaia Carroll
  • , Ritika Dusad
  • , Jonathan Ward
  • , Catherine Dawson
  • , Sudarshan Sharma
  • , Graeme M. Luke
  • , Stephen J. Blundell
  • , Claudio Castelnovo
  • , Jonathan N. Hallén
  • , Roderich Moessner
  • , J. C.Séamus Davis
  • University of Oxford
  • Max Planck Institute for Chemical Physics of Solids
  • University College Cork
  • McMaster University
  • University of Cambridge
  • Max-Planck-Institute for the Physics of Complex Systems
  • Cornell University

Research output: Contribution to journalArticlepeer-review

Abstract

A recent advance in the study of emergent magnetic monopoles was the discovery that monopole motion is restricted to dynamical fractal trajectories [J. N. Hallén et al., Science 378, 1218 (2022)], thus explaining the characteristics of magnetic monopole noise spectra [R. Dusad et al., Nature 571, 234 (2019); A. M. Samarakoon et al., Proc. Natl. Acad. Sci. U.S.A. 119, e2117453119 (2022)]. Here, we apply this novel theory to explore the dynamics of field-driven monopole currents, finding them composed of two quite distinct transport processes: initially swift fractal rearrangements of local monopole configurations followed by conventional monopole diffusion. This theory also predicts a characteristic frequency dependence of the dissipative loss angle for AC field–driven currents. To explore these novel perspectives on monopole transport, we introduce simultaneous monopole current control and measurement techniques using SQUID-based monopole current sensors. For the canonical material Dy2Ti2O7, we measure Φ(t), the time dependence of magnetic flux threading the sample when a net monopole current J(t) = Φ̇(t)∕μ0 is generated by applying an external magnetic field B0(t). These experiments find a sharp dichotomy of monopole currents, separated by their distinct relaxation time constants before and after t ~600 μs from monopole current initiation. Application of sinusoidal magnetic fields B0(t) = Bcos(ωt) generates oscillating monopole currents whose loss angle θ(f )exhibits a characteristic transition at frequency f ≈ 1.8 kHz over the same temperature range. Finally, the magnetic noise power is also dichotomic, diminishing sharply after t ~600 μs. This complex phenomenology represents an unprecedented form of dynamical heterogeneity generated by the interplay of fractionalization and local spin configurational symmetry.

Original languageEnglish
Article numbere2320384121
JournalProceedings of the National Academy of Sciences of the United States of America
Volume121
Issue number21
DOIs
Publication statusPublished - 2024

Keywords

  • dysprosium titanate
  • frustrated magnetism
  • magnetic dynamics
  • spin ice

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