TY - JOUR
T1 - Visualizing the atomic-scale origin of metallic behavior in Kondo insulators
AU - Pirie, Harris
AU - Mascot, Eric
AU - Matt, Christian E.
AU - Liu, Yu
AU - Chen, Pengcheng
AU - Hamidian, M. H.
AU - Saha, Shanta
AU - Wang, Xiangfeng
AU - Paglione, Johnpierre
AU - Luke, Graeme
AU - Goldhaber-Gordon, David
AU - Hirjibehedin, Cyrus F.
AU - Davis, J. C.Séamus
AU - Morr, Dirk K.
AU - Hoffman, Jennifer E.
N1 - Publisher Copyright:
© 2023 American Association for the Advancement of Science. All rights reserved.
PY - 2023/3/24
Y1 - 2023/3/24
N2 - A Kondo lattice is often electrically insulating at low temperatures. However, several recent experiments have detected signatures of bulk metallicity within this Kondo insulating phase. In this study, we visualized the real-space charge landscape within a Kondo lattice with atomic resolution using a scanning tunneling microscope. We discovered nanometer-scale puddles of metallic conduction electrons centered around uranium-site substitutions in the heavy-fermion compound uranium ruthenium silicide (URu2Si2) and around samarium-site defects in the topological Kondo insulator samarium hexaboride (SmB6). These defects disturbed the Kondo screening cloud, leaving behind a fingerprint of the metallic parent state. Our results suggest that the three-dimensional quantum oscillations measured in SmB6 arise from Kondo-lattice defects, although we cannot exclude other explanations. Our imaging technique could enable the development of atomic-scale charge sensors using heavy-fermion probes.
AB - A Kondo lattice is often electrically insulating at low temperatures. However, several recent experiments have detected signatures of bulk metallicity within this Kondo insulating phase. In this study, we visualized the real-space charge landscape within a Kondo lattice with atomic resolution using a scanning tunneling microscope. We discovered nanometer-scale puddles of metallic conduction electrons centered around uranium-site substitutions in the heavy-fermion compound uranium ruthenium silicide (URu2Si2) and around samarium-site defects in the topological Kondo insulator samarium hexaboride (SmB6). These defects disturbed the Kondo screening cloud, leaving behind a fingerprint of the metallic parent state. Our results suggest that the three-dimensional quantum oscillations measured in SmB6 arise from Kondo-lattice defects, although we cannot exclude other explanations. Our imaging technique could enable the development of atomic-scale charge sensors using heavy-fermion probes.
UR - https://www.scopus.com/pages/publications/85150911735
U2 - 10.1126/science.abq5375
DO - 10.1126/science.abq5375
M3 - Article
C2 - 36952423
AN - SCOPUS:85150911735
SN - 0036-8075
VL - 379
SP - 1214
EP - 1218
JO - Science
JF - Science
IS - 6638
ER -